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d1292d8 | 1 2 3 4 5 6 7 8 9 10 11 12 13 14 15 16 17 18 19 20 21 22 23 24 25 26 27 28 29 30 31 32 33 34 35 36 37 38 39 40 41 42 43 44 45 46 47 48 49 50 51 52 53 54 55 56 57 58 59 60 61 62 63 64 65 66 67 68 69 70 71 72 73 74 75 76 77 78 79 80 81 82 83 84 85 86 87 88 89 90 91 92 93 94 95 96 97 98 99 100 101 102 103 104 105 106 107 108 109 110 111 112 113 114 115 116 117 118 119 120 121 122 123 124 125 126 127 128 129 130 131 132 133 134 135 136 137 138 139 140 141 142 143 144 145 146 147 148 149 150 151 152 153 154 155 156 157 158 159 160 161 162 163 164 165 166 167 168 169 170 171 172 173 174 175 176 177 178 179 180 181 182 183 184 185 186 187 188 189 190 191 192 193 194 195 196 197 198 199 200 201 202 203 204 205 206 207 208 209 210 211 212 213 214 215 216 217 | """Template-backed static-headspace path for the Agilent 8697 runtime (CHEM-108).
Library: ``assets/reactions/agilent_hs8697_headspace_library/templates.json`` — Sander (2023) measured Henry
solubility constants Hscp = c_aq / p (water, infinite dilution, 298.15 K) with the temperature coefficient
B = -d ln Hscp / d(1/T) where published (68 of 77 spectral_library compounds).
Physics for a sealed vial with an aqueous sample (two-phase closed system at equilibrium):
Hscp(T) = Hscp(298.15) * exp(B (1/T - 1/298.15))
K(T) = c_liquid / c_gas = Hscp(T) * R * T (dimensionless partition coefficient)
beta = V_gas / V_liquid (phase ratio)
c_gas = c0 / (K + beta) (mass balance c0 V_L = c_L V_L + c_G V_G)
The headspace transferred to the GC is c_gas x loop volume (host-declared assumption, the vendor loop volume is
unknown) and is chromatographed with the 8890B template GC model (spectral_library/gc_retention.json fingerprints).
"""
from __future__ import annotations
import copy
import json
import math
from typing import Any
from scripts.basic40_templates import _analytical_common as common
from scripts.basic40_templates import agilent_gc8890b as gc_templates
from scripts.template_library import get_template, index_by_id
LIB_REL = "assets/reactions/agilent_hs8697_headspace_library/templates.json"
R = 8.31446261815324
T_REF = 298.15
T_REF_TOLERANCE_K = 0.5
MAX_SPECIES = 16
MAX_INITIAL_CONCENTRATION_MOL_M3 = 100.0 # 0.1 mol/L: keep the infinite-dilution Henry law plausible
VIAL_VOLUMES_M3 = (10e-6, 20e-6, 22e-6)
LIMITATIONS = [
"Sander (2023) Henry constants are for pure water at infinite dilution; salting-out, co-solvents, matrix effects, non-ideal (concentrated) solutions and adsorption on vial/septum are not modelled.",
"Temperature dependence uses the published van 't Hoff coefficient B; records without B are usable only at 298.15 +/- 0.5 K (no extrapolation). Extrapolation of B to headspace oven temperatures far above 298 K is itself an approximation.",
"Complete equilibrium is assumed at the oven setpoint; the configured equilibration time is not used to model mass-transfer kinetics, and shaking/pressurization are not modelled.",
"Loop volume and GC method of the transfer are trusted-host assumptions (the 8697 loop volume is unknown); vial pressurization/dilution of the loop gas is ignored.",
"The chromatogram uses the 8890B template GC model (NIST retention indices -> derived fingerprints with an assumed column calibration); species without a GC fingerprint for the selected column are transferred but not chromatographed.",
"Selection of one Sander record per compound is transparent (M-type closest to the median of all M-type values) but is not a new critical evaluation; alternatives are summarised in the library.",
]
SYNTHETIC_PARTS = ["loop volume (host assumption)", "GC transfer method (host assumption)"] + gc_templates.SYNTHETIC_PARTS
def _resolve(identifier: Any) -> str | None:
if not isinstance(identifier, str) or not identifier:
return None
index = index_by_id(LIB_REL)
if identifier in index:
return identifier
for sid, record in index.items():
if identifier in (record.get("shared_ids") or {}).values():
return sid
return None
def henry_at(record: dict[str, Any], temperature_K: float) -> float | None:
"""Hscp(T) [mol m^-3 Pa^-1] or None when T is outside the record's usable range."""
b = record["henry_temperature_coefficient_K"]
if b is None:
return record["henry_hscp_mol_m3_pa"] if abs(temperature_K - T_REF) <= T_REF_TOLERANCE_K else None
return record["henry_hscp_mol_m3_pa"] * math.exp(b * (1.0 / temperature_K - 1.0 / T_REF))
def template_read(substance_id: Any) -> dict[str, Any] | None:
sid = _resolve(substance_id)
record = get_template(LIB_REL, sid) if sid else None
if record is None:
return None
return {"substance_id": sid, "name": record["name"], "name_zh": record["name_zh"], "cas": record["cas"],
"molar_mass_kg_mol": record["molar_mass_kg_mol"], "henry_hscp_mol_m3_pa": record["henry_hscp_mol_m3_pa"],
"henry_temperature_coefficient_K": record["henry_temperature_coefficient_K"], "reference_temperature_K": T_REF,
"partition_coefficient_K_298": record["partition_coefficient_K_298"],
"alternatives_measured": record["alternatives_measured"], "conditions_json": json.dumps(record["conditions"], ensure_ascii=False),
"source": record["source"], "gc_retention_id": record["gc_link"]["gc_retention_id"],
**common.provenance([LIB_REL], record["evidence"] + " (Hscp, B); K_298 derived = Hscp*R*T", SYNTHETIC_PARTS, LIMITATIONS)}
def validate_sample(composition_mol_m3: Any, *, liquid_volume_m3: float, vial_volume_m3: float) -> dict[str, Any]:
if vial_volume_m3 not in VIAL_VOLUMES_M3:
raise ValueError("vial volume must be 10/20/22 mL in m^3")
if not common.finite(liquid_volume_m3) or not 0 < liquid_volume_m3 < vial_volume_m3:
raise ValueError("liquid_volume_m3 must be positive and smaller than the vial volume (a headspace is required)")
if not isinstance(composition_mol_m3, dict) or not 1 <= len(composition_mol_m3) <= MAX_SPECIES:
raise ValueError(f"composition_mol_m3 must map 1..{MAX_SPECIES} library ids to initial aqueous mol/m^3")
out = {}
for identifier, concentration in composition_mol_m3.items():
sid = _resolve(identifier)
if sid is None:
raise ValueError(f"{identifier!r} has no Henry record in {LIB_REL}")
if sid in out:
raise ValueError(f"duplicate compound {sid!r}")
if not common.finite(concentration) or not 0 < concentration <= MAX_INITIAL_CONCENTRATION_MOL_M3:
raise ValueError(f"initial concentration for {identifier!r} must be in (0, {MAX_INITIAL_CONCENTRATION_MOL_M3}] mol/m^3")
out[sid] = float(concentration)
return {"library": LIB_REL, "composition_mol_m3": out, "liquid_volume_m3": float(liquid_volume_m3),
"vial_volume_m3": float(vial_volume_m3), "solvent": "water"}
def validate_transfer(*, loop_volume_m3: float, gc_column: str = "nonpolar", gc_oven_temperature_K: float = 353.15,
gc_inlet_temperature_K: float = 523.15, gc_fid_temperature_K: float = 573.15,
split_ratio: float = 20.0) -> dict[str, Any]:
if not common.finite(loop_volume_m3) or not 1e-8 <= loop_volume_m3 <= 1e-5:
raise ValueError("loop_volume_m3 must be within 0.01..10 mL (host assumption)")
if gc_column not in gc_templates.COLUMNS:
raise ValueError("gc_column must be nonpolar or polar")
for value in (gc_oven_temperature_K, gc_inlet_temperature_K, gc_fid_temperature_K):
if not common.finite(value) or not 273.15 <= value <= 723.15:
raise ValueError("GC temperatures must be within 273.15..723.15 K")
if gc_fid_temperature_K < gc_templates.FID_IGNITION_MINIMUM_K:
raise ValueError("FID temperature below the gc_runtime ignition minimum")
if not common.finite(split_ratio) or not 0 < split_ratio <= 1000:
raise ValueError("split_ratio must be in (0, 1000]")
return {"loop_volume_m3": float(loop_volume_m3), "gc_column": gc_column, "gc_oven_temperature_K": float(gc_oven_temperature_K),
"gc_inlet_temperature_K": float(gc_inlet_temperature_K), "gc_fid_temperature_K": float(gc_fid_temperature_K),
"split_ratio": float(split_ratio), "evidence": "assumption"}
def equilibrium(template: dict[str, Any], temperature_K: float, loop_volume_m3: float | None = None) -> dict[str, Any] | None:
"""Per-species equilibrium headspace (trusted-host detail); None if any species lacks data at temperature_K."""
beta = (template["vial_volume_m3"] - template["liquid_volume_m3"]) / template["liquid_volume_m3"]
species = {}
for sid, c0 in template["composition_mol_m3"].items():
record = get_template(LIB_REL, sid)
hscp = henry_at(record, temperature_K)
if hscp is None:
return None
k = hscp * R * temperature_K
c_gas = c0 / (k + beta)
entry = {"henry_hscp_mol_m3_pa": hscp, "partition_coefficient_K": k, "gas_concentration_mol_m3": c_gas,
"liquid_concentration_mol_m3": k * c_gas, "partial_pressure_pa": c_gas * R * temperature_K,
"fraction_in_gas": c_gas * beta / c0, "molar_mass_kg_mol": record["molar_mass_kg_mol"],
"gc_retention_id": record["gc_link"]["gc_retention_id"]}
if loop_volume_m3 is not None:
entry["loop_mol"] = c_gas * loop_volume_m3
entry["loop_mass_kg"] = c_gas * loop_volume_m3 * record["molar_mass_kg_mol"]
species[sid] = entry
return {"temperature_K": temperature_K, "phase_ratio": beta, "vial_volume_m3": template["vial_volume_m3"],
"liquid_volume_m3": template["liquid_volume_m3"], "loop_volume_m3": loop_volume_m3, "species": species}
def measure(template: dict[str, Any], transfer: dict[str, Any] | None, oven_temperature_K: float,
equilibration_time_s: float | None) -> dict[str, Any] | None:
"""Agent-visible result for a template-backed vial; None when a precondition of the template path fails."""
if transfer is None:
return None
eq = equilibrium(template, oven_temperature_K, transfer["loop_volume_m3"])
if eq is None:
return None
composition = {sid: item["loop_mass_kg"] for sid, item in eq["species"].items()
if item["gc_retention_id"] and gc_templates.fingerprint(sid, transfer["gc_column"]) and item["loop_mass_kg"] > 0}
if not composition:
return None
gc_template = gc_templates.validate_sample(composition, column=transfer["gc_column"], injection_fraction=1.0)
run = gc_templates.simulate(gc_template, oven_K=transfer["gc_oven_temperature_K"], inlet_K=transfer["gc_inlet_temperature_K"],
fid_K=transfer["gc_fid_temperature_K"], split_ratio=transfer["split_ratio"])
if run is None:
return None
return {"chromatogram": run["public"],
"headspace": {"oven_temperature_K": oven_temperature_K, "vial_volume_m3": eq["vial_volume_m3"],
"phase_ratio": eq["phase_ratio"], "loop_volume_m3": transfer["loop_volume_m3"],
"equilibration_time_s": equilibration_time_s, "equilibrium_assumed": True,
"gc_column_model": transfer["gc_column"], "gc_oven_temperature_K": transfer["gc_oven_temperature_K"],
"split_ratio": transfer["split_ratio"]},
**common.provenance([LIB_REL, gc_templates.LIB_REL],
"Henry constants: Sander 2023 measured_literature; partition/transfer: derived; GC: NIST RI -> derived fingerprints",
SYNTHETIC_PARTS, LIMITATIONS)}
def result_schema() -> dict[str, Any]:
n, obj, nullable = common.number, common.obj, common.nullable
headspace = obj({"oven_temperature_K": n("K", 0), "vial_volume_m3": n("m3", 0), "phase_ratio": n("1", 0),
"loop_volume_m3": n("m3", 0), "equilibration_time_s": nullable(n("s", 0)),
"equilibrium_assumed": {"type": "boolean", "const": True},
"gc_column_model": {"type": "string", "enum": list(gc_templates.COLUMNS)},
"gc_oven_temperature_K": n("K", 0), "split_ratio": n("1", 0)})
return obj({"chromatogram": gc_templates.chromatogram_schema(), "headspace": headspace, **common.provenance_schema()})
def template_read_schema() -> dict[str, Any]:
n, obj, nullable = common.number, common.obj, common.nullable
alternatives = obj({"n": {"type": "integer", "minimum": 1, "x-unit": "1"}, "n_with_temperature_coefficient": {"type": "integer", "minimum": 0, "x-unit": "1"},
"hscp_median": n("mol/(m^3*Pa)", 0), "hscp_min": n("mol/(m^3*Pa)", 0), "hscp_max": n("mol/(m^3*Pa)", 0)})
return obj({"substance_id": common.TEXT, "name": common.TEXT, "name_zh": common.TEXT, "cas": nullable(common.TEXT),
"molar_mass_kg_mol": n("kg/mol", 0), "henry_hscp_mol_m3_pa": n("mol/(m^3*Pa)", 0),
"henry_temperature_coefficient_K": nullable(n("K")), "reference_temperature_K": n("K", 0),
"partition_coefficient_K_298": n("1", 0), "alternatives_measured": alternatives, "conditions_json": common.TEXT,
"source": common.TEXT, "gc_retention_id": nullable(common.TEXT), **common.provenance_schema()})
def extend_metadata(metadata: dict[str, Any]) -> dict[str, Any]:
caps, slots = metadata["capabilities"], metadata["state_slots"]
legacy_output = caps["measure"]["output_schema"]
caps["measure"]["output_schema"] = {"anyOf": [legacy_output, result_schema()]}
caps["measure"]["preconditions"] = caps["measure"]["preconditions"] + [
"Template-backed vial only: host configure_template_transfer() done; every species has Henry data at the oven setpoint (B published, or setpoint 298.15 +/- 0.5 K); at least one species has a GC fingerprint."]
legacy_chromatogram = slots["measurement.chromatogram"]["value_schema"]["anyOf"][0]
slots["measurement.chromatogram"]["value_schema"] = {"anyOf": [legacy_chromatogram, gc_templates.chromatogram_schema(), {"type": "null"}]}
log_item = slots["injection.log"]["value_schema"]["items"]
template_log = copy.deepcopy(log_item)
template_log["properties"]["synthetic"] = {"type": "boolean", "const": False}
slots["injection.log"]["value_schema"]["items"] = {"anyOf": [log_item, template_log]}
status = slots["vial.status"]["value_schema"]["items"]["properties"]["status"]
status["enum"] = status["enum"] + ["measured_template"]
cap = common.template_read_capability(
"AgilentHS8697", "toluene", template_read_schema(), ["display"],
"Henry-law library id (spectral_library compound id); does not refer to any loaded vial")
cap["errors"] = ["UNKNOWN_INSTANCE", "UNKNOWN_CAPABILITY", "INVALID_ARGUMENT", "REQUEST_CONFLICT"]
caps["template.read"] = cap
metadata["parameters"]["template_library"] = {"value": LIB_REL, "unit": "1", "evidence": "measured_literature",
"conditions": "Sander (2023) Henry solubility constants, water, infinite dilution; 68/77 with temperature coefficient"}
metadata["parameters"]["template_loop_volume_m3"] = {"value": None, "unit": "m3", "evidence": "unknown",
"conditions": "Must be declared by the trusted host via configure_template_transfer(loop_volume_m3=..., evidence='assumption')"}
metadata["limits"] = metadata["limits"] + [
"Template-backed vials (host register_template_sample + configure_template_transfer) use Henry-law partition K(T) and phase ratio to compute the headspace and chromatograph it with the 8890B template GC model; the synthetic fixture path is unchanged and remains the default."]
return metadata
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