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arxiv:2610.05714

Current selects the helicity of a chiral phonon

Published on Oct 5
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Abstract

A DC bias in chiral conductors breaks phonon helicity symmetry, generating net lattice chirality and self-sustained traveling waves without optical pumping.

The emergence of spin-polarized electrons from nonmagnetic chiral molecules and crystals is called Chirality-induced spin selectivity (CISS). A chiral phonon of definite wavevector q can strongly enhance it, but near equilibrium the two helicities +q and -q are equally populated: they are time-reversal partners and their contributions cancel. We show that in a biased chiral conductor the current causes the phonon of one helicity to damp less than the other. The damping asymmetry is odd in the current, odd under qrightarrow-q, invariant under a mirror that reverses the structural handedness, and equal, mode for mode, to the current-induced nonconservative Berry force on the phonon coordinate. Closing the phonon kinetics with a rate equation turns the asymmetry into a net lattice helicity: at any finite bias one helicity is preferentially populated, with no threshold, growing linearly with the current as Vrightarrow0; above a threshold that helicity becomes a self-sustained coherent travelling wave. We demonstrate this effect in elemental tellurium, treated as an open quantum system (electronic Hamiltonian, phonon bath, and electron-phonon coupling) within a quasi-ab initio framework. The electronic Hamiltonian is supplied by a vertex-corrected quasiparticle self-consistent GW (QSGW) potential with spin-orbit coupling; nuclear displacements are modeled with a machine-learned interatomic potential, which yields chiral phonon modes at finite pm q_z on the Γ-A line. The perturbation to the electronic Hamiltonian from a nuclear displacement is approximated by a frozen-phonon deformation potential. No optical pump is needed: a bias alone drives the current and selects the phonon helicity; reversing the current reverses the selection.

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